Deciphering mass transport behavior in membrane electrode assembly by manipulating porous structures of atomically dispersed Metal-Nx catalysts for High-Efficiency electrochemical CO2 conversion > Journals

Author: Seunghyun Lee, Ye Eun Jeon, Seonggyu Lee, Wonhee Lee, Seongbeen Kim, Jaeryung Choi, Jinkyu Park, Jeong Woo Han, You Na Ko, Young Eun Kim, Jinwon Park, Jungbae Kim*, Ki Tae Park*, Jinwoo Lee*

• A systematic study for the effect of porous structures on CO production was performed.

• Different performance trends between H-cell and full cell analyses were observed.

• A thin catalyst layer possessing mesopores promoted CO production in MEA condition.

• The optimized catalyst exhibited the highest energy efficiency (55 %) at 265 mA cm−1.